Weak temperature dependence of ageing of structural properties in atomistic model glassformers

We have just published in the Journal of Chemical Physics the simulation work of a brilliant former master student of the School of Physics at the University of Bristol (Thomas Jenkinson) on the local structural changes occurring during ageing in two atomistic glass formers with Lennard-Jones interactions (the Kob-Andersen and Wahnström mixtures).

We find some expected results (local order steadily increases as the out-of-equilibrium liquid ages) and some more surprising ones (for example, the rate at which such increase occurs changes weakly for temperatures above the apparent dynamical divergence of viscosities, T0). We also investigate the effect of transient deep quenches, finding very moderate traces of so-called rejuvenation.

The reference to the work is J. Chem. Phys. 147, 054501, (2017).

Published by

francescoturci

Physicist and oboe player.

Leave a Reply

Fill in your details below or click an icon to log in:

WordPress.com Logo

You are commenting using your WordPress.com account. Log Out /  Change )

Twitter picture

You are commenting using your Twitter account. Log Out /  Change )

Facebook photo

You are commenting using your Facebook account. Log Out /  Change )

Connecting to %s